First, currently-known color centers either exhibit long spin coherence times or efficient, coherent optical transitions, but not both. We have developed new methods to control the diamond Fermi level in order to stabilize a new color center, the neutral charge state of the silicon vacancy (SiV) center, which exhibits both the excellent optical properties of the negatively charged SiV center and the long spin coherence times of the NV center, making it a promising candidate for applications as a single atom quantum memory for long distance quantum communication.
Second, color centers placed close to the diamond surface can have strong interactions with molecules and materials external to the diamond. However, uncontrolled surface termination and contamination can degrade the color center properties and give rise to noise that obscures the signal of interest. I will describe our recent efforts to stabilize shallow NV centers within 5 nm of the surface using new surface processing and termination techniques. These highly coherent, shallow NV centers will provide a platform for sensing and imaging down to the scale of single atoms.