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R. G. Herb Condensed Matter Seminar
Dynamical breaking of inversion symmetry, strong second harmonic generation, and ferroelectricity with nonlinear phonons
Date: Thursday, March 5th
Time: 10:00 am - 11:00 am
Place: 5310 Chamberlin Hall
Speaker: Egor Kiselev , MPIPKS
Abstract: I will show how crystalline inversion symmetry can be dynamically broken by optical phonons with generic, hardening Kerr-like non-linearities. The symmetry-broken state is reached through a dynamical phase transition that can be accessed by driving close to half the phonon resonance. After going through an instability, the system settles to a steady state with inversion-symmetry breaking phonon trajectories and strong second harmonic generation. The time averaged positions of the atoms are displaced relative to equilibrium, resulting in a rectification of the driving signal. This leads to a dynamical dipolar, ferroelectric response that shows features like hysteresis and memory effects, known from equilibrium ferroelectrics.
Host: Elio König
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